Local structure and polaron formation in Lal_xCaxMnO3

ثبت نشده
چکیده

The local structure of La 1 .~Ca~MnO 3 is determined from pair-distribution function (PDF) analysis of pulsed neutron diffraction. We have compared the effect on the local structure of crossing the metal-insulator transition as a function of temperature and composition. Crossing the metal insulator boundary at low temperature by varying the composition yields similar distortions to those seen in the temperature dependence indicating the presence of polarons in the insulating phase which disappear in the metallic phase. ~', 1998 Published by Elsevier Science B.V. All rights reserved.

برای دانلود متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

ثبت نام

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

منابع مشابه

Spin-lattice Correlations and Temperature Dependent Mn JT-edge Structure in the Lai_xCaxMnO3 Systems

The Lai^Ca^MnOs system exhibits novel transport properties and unusual correlations between local distortions, magnetism, and the electronic structure. A large distortion, parameterized by the width of the pair distribution function, a, develops as T is increased through Tc for values of jc roughly from 0.2-0.5 (the colossal magnetoresistance (CMR) regime); we associate this change of the local...

متن کامل

Localisation versus self-trapping: Polaron formation in the Anderson-Holstein model

The polaron concept, first introduced by Landau [1], is one of the main pillars on which the theoretical analysis of materials with strong electron-phonon (EP) coupling rests. In these compounds, the coupling between the electron and the lattice leads to a lattice deformation whose potential tends to bind the electron to the deformed region of the crystal. This process, which has been called se...

متن کامل

Temperature dependent evolution of the electronic and local atomic structure in the cubic colossal magnetoresistive manganite La1-xSrxMnO3

We have studied the temperature-dependent evolution of the electronic and local atomic structure in the cubic colossal magnetoresistive manganite La1-xSrxMnO3 (x= 0.3 – 0.4) with core and valence level photoemission (PE), x-ray absorption specroscopy (XAS), x-ray emission spectroscopy (XES), resonant inelastic x-ray scattering (RIXS), extended x-ray absorption fine structure (EXAFS) spectroscop...

متن کامل

Ferromagnetism and Transport in the Double-Exchange Model, with and without Phonons; Application to the Manganites

An introduction is given to the many-body coherent potential approximation (CPA) for the double-exchange (DE) model and the Holstein-DE model, the latter including coupling of the electrons to local phonons as well as to the local spins. It is shown how the method can treat the local spins and phonons quantum-mechanically and how it is equivalent to dynamical mean field theory in the classical ...

متن کامل

Electric pulse induced resistance change effect in manganites due to polaron localization at the metal-oxide interfacial region

Combining pulse-probe measurements as well as local transport measurements in an electron microscope system by a simultaneous monitoring of the structural changes, we show that the nonvolatile electric pulse induced resistance change in Ca-doped praseodymium manganite is related to a polaron order-disorder transition, modified by electronic band bending in the vicinity of an interface to a meta...

متن کامل

ذخیره در منابع من


  با ذخیره ی این منبع در منابع من، دسترسی به آن را برای استفاده های بعدی آسان تر کنید

برای دانلود متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

ثبت نام

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

عنوان ژورنال:

دوره   شماره 

صفحات  -

تاریخ انتشار 2002